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Unseen in the air around us are tiny molecules that drive the chemical cocktail of our atmosphere. As plants, animals, volcanoes, wildfires and human activities spew particles into the atmosphere, som...
The reactive uptake of carbonyl-containing volatile organic compounds (cVOCs) by aqueous atmospheric aerosols is a likely source of particulate organic material. The aque ous-phase secondary organic p...
Reactive nitrogen compounds, specifically NOx and NO3, likely influence global organic aerosol levels. To assess these interactions, GEOS-Chem, a chemical transport model, is updated to include improv...
A large dataset of reactive trace gases was collected for the first time over West Africa during the African Monsoon Multidisciplinary Analysis (AMMA) field experiment in August 2006. Volatile Organic...
Emissions from major point sources are badly represented by classical Eulerian models. An overestimation of the horizontal plume dilution, a bad representation of the vertical diffusion as well as an ...
We interpret observations from the Intercontinental Chemical Transport Experiment, Phase B (INTEX-B) in spring 2006 using a global chemical transport model (GEOS-Chem) to evaluate sensitivities of the...
We present and discuss a new dataset of gridded emissions covering the historical period (1850–2000) in decadal increments at a horizontal resolution of 0.5° in latitude and longitude. The primary pur...
Although tropospheric reactive halogen chemistry is well studied in coastal and polar environments, the presence of halogens over the open ocean environment has not been widely reported. The impacts o...
Atmospheric mercury species concentrations were measured during two oceanographic cruise campaigns covering the Adriatic Sea, the first during the autumn in 2004 and the second in the summer of 2005. ...
This paper presents a summary of the measurements made during the heavily-instrumented Reactive Halogens in the Marine Boundary Layer (RHaMBLe) coastal study in Roscoff on the North West coast of Fran...
We present investigations of the reactive iodine species (RIS) IO, OIO and I2 in a coastal region from a field campaign simultaneously employing active long path differential optical absorption spectr...
The NERC UK SOLAS-funded Reactive Halogens in the Marine Boundary Layer (RHaMBLe) programme comprised three field experiments. This manuscript presents an overview of the measurements made within the ...
Atmospheric concentrations of the volatile reactive iodocarbons C2H5I, 1-C3H7I, 2-C3H7I, CH2ICl, CH2IBr, CH2I2 and bromocarbons CH2Br2 and CHBr3 were determined by GC/MS analysis of marine boundary la...
The nitrogen (δ15N) and triple oxygen (δ17O and δ18O) isotopic composition of nitrate (NO3−) was measured year-round in the atmosphere and snow pits at Dome C, Antarctica (DC, 75.1° S, 123.3° E)...
The chemical cycling and spatiotemporal distribution of mercury in the troposphere is poorly understood. We measured gaseous elemental mercury (GEM), reactive gaseous mercury (RGM) and particulate mer...

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