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氧化亚氮(N2O)、甲烷(CH4)和二氧化碳(CO2)是大气中最重要的三种温室气体。基于湍流理论的涡动相关法是测量地气间温室气体交换通量的理想方法,该方法对生态系统干扰小,并可获得长时间序列的观测数据。然而,目前现有的基于涡动相关法的观测设备只能有效测量上述三种气体中的一种或至多两种气体的通量。王凯、王东(博士生)和郑循华所在的碳氮循环团队采用一台闭路量子级联激光(QCL)气体分析仪和相关设备配件...
Absorption cross sections of nitrous oxide (N2O) and carbon tetrachloride (CCl4) are reported at five atomic UV lines (184.95, 202.548, 206.200, 213.857, and 228.8 nm) at temperatures in the range 210...
Nitrous oxide (N2O) is the third most important anthropogenic greenhouse gas. Globally, the main sources of N2O are nitrification and denitrification in soils. About two thirds of the soil emissions o...
An open-top-chamber (OTC) CO2 enrichment (~720 mmol mol-1) study was conducted in the Colorado shortgrass steppe from April 1997 through October 2001. Aboveground plant biomass increased under elevate...
We have performed high-precision measurements of the 18O and position dependent 15N isotopic composition of N2O from Antarctic firn air samples. By comparing these data to simulations carried out with...
CO, CH4, N2O and CO2 were retrieved from high resolution solar absorption spectra obtained during a ship cruise from Capetown to Bremerhaven in January/February 2003 by Fourier Transform Infrared (FTI...
In this paper we study the impact of the modelling of N2O on the simulation of NO2 and HNO3 by comparing in situ vertical profiles measured at mid-latitudes with the results of the Reprobus 3-D CTM (T...
We present measurements of NO, NOy, O3, and N2O within the lowermost stratosphere (LMS) over Europe obtained during the SPURT project. The measurements cover all seasons between November 2001 and Jul...
The absolute rate constant for the reaction that is the major source of stratospheric NOx, O(1D)+N2O → products, has been determined in the temperature range 227 K to 719 K, and, in the temperature ra...
N2O abundances ranging from 0.5 to 6 ppbv were observed in the polar upper stratosphere/lower mesosphere by the MIPAS instrument on the Envisat satellite during the Arctic and Antarctic winters in the...

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